The performance of battery materials is determined by their composition and the processing conditions employed during commercial-scale fabrication, where raw materials undergo complex processing steps with various additives to yield final products. As the complexity of these parameters expands with the development of industry, conventional one-factor-at-a-time (OFAT) experiment becomes old fashioned. While domain expertise aids in parameter optimization, this traditional approach becomes increasingly vulnerable to cognitive limitations and anthropogenic biases as the complexity of factors grows. Herein, we introduce an iterative machine learning (ML) framework that integrates active learning to guide targeted experimentation and facilitate incremental model refinement. This method systematically leverages comprehensive experimental observations, including both successful and unsuccessful results, effectively mitigating human-induced biases and alleviating data scarcity. Consequently, it significantly accelerates exploration within the high-dimensional design space. Our results demonstrate that active-learning-driven experimentation markedly reduces the total number of experimental cycles necessary, underscoring the transformative potential of ML-based strategies in expediting battery material optimization.

Accurate prediction of lithium-ion battery lifespan is vital for ensuring operational reliability and reducing maintenance costs in applications like electric vehicles and smart grids. This study presents a hybrid learning framework for precise battery lifespan prediction, integrating dynamic multi-source data fusion with a stacked ensemble (SE) modeling approach. By leveraging heterogeneous datasets from the National Aeronautics and Space Administration (NASA), Center for Advanced Life Cycle Engineering (CALCE), MIT-Stanford-Toyota Research Institute (TRC), and nickel cobalt aluminum (NCA) chemistries, an entropy-based dynamic weighting mechanism mitigates variability across heterogeneous datasets. The SE model combines Ridge regression, long short-term memory (LSTM) networks, and eXtreme Gradient Boosting (XGBoost), effectively capturing temporal dependencies and nonlinear degradation patterns. It achieves a mean absolute error (MAE) of 0.0058, root mean square error (RMSE) of 0.0092, and coefficient of determination (R2) of 0.9839, outperforming established baseline models with a 46.2% improvement in R2 and an 83.2% reduction in RMSE. Shapley additive explanations (SHAP) analysis identifies differential discharge capacity (Qdlin) and temperature of measurement (Temp_m) as critical aging indicators. This scalable, interpretable framework enhances battery health management, supporting optimized maintenance and safety across diverse energy storage systems, thereby contributing to improved battery health management in energy storage systems.

Accurate prediction of the Remaining Useful Life (RUL) in Lithium ion battery (LIB) health management systems is essential for ensuring operational reliability and safety. However, many existing methods assume that training and testing data follow the same distribution, limiting their ability to generalize to unseen target domains. To address this, we propose a novel RUL prediction framework that incorporates a domain adaptation (DA) technique. Our framework integrates a signal preprocessing pipeline including noise reduction, feature extraction, and normalization with a robust deep learning model called HybridoNet Adapt. The model features a combination of LSTM, Multihead Attention, and Neural ODE layers for feature extraction, followed by two predictor modules with trainable trade-off parameters. To improve generalization, we adopt a DA strategy inspired by Domain Adversarial Neural Networks (DANN), replacing adversarial loss with Maximum Mean Discrepancy (MMD) to learn domain-invariant features. Experimental results show that HybridoNet Adapt significantly outperforms traditional models such as XGBoost and Elastic Net, as well as deep learning baselines like Dual input DNN, demonstrating its potential for scalable and reliable battery health management (BHM).

Health evaluation for lithium-ion batteries (LIBs) typically relies on constant charging/discharging protocols, often neglecting scenarios involving dynamic current profiles prevalent in electric vehicles. Conventional health indicators for LIBs also depend on the uniformity of measured data, restricting their adaptability to non-uniform conditions. In this study, a novel training strategy for estimating LIB health based on the paradigm of self-supervised learning is proposed. A multiresolution analysis technique, empirical wavelet transform, is utilized to decompose non-stationary voltage signals in the frequency domain. This allows the removal of ineffective components for the health evaluation model. The transformer neural network serves as the model backbone, and a loss function is designed to describe the capacity degradation behavior with the assumption that the degradation in LIBs across most operating conditions is inevitable and irreversible. The results show that the model can learn the aging characteristics by analyzing sequences of voltage and current profiles obtained at various time intervals from the same LIB cell. The proposed method is successfully applied to the Stanford University LIB aging dataset, derived from electric vehicle real driving profiles. Notably, this approach achieves an average correlation coefficient of 0.9 between the evaluated health index and the degradation of actual capacity, demonstrating its efficacy in capturing LIB health degradation. This research highlights the feasibility of training deep neural networks using unlabeled LIB data, offering cost-efficient means and unleashing the potential of the measured information.

As the use of Lithium-ion batteries continues to grow, it becomes increasingly important to be able to predict their remaining useful life. This work aims to compare the relative performance of different machine learning algorithms, both traditional machine learning and deep learning, in order to determine the best-performing algorithms for battery cycle life prediction based on minimal data. We investigated 14 different machine learning models that were fed handcrafted features based on statistical data and split into 3 feature groups for testing. For deep learning models, we tested a variety of neural network models including different configurations of standard Recurrent Neural Networks, Gated Recurrent Units, and Long Short Term Memory with and without attention mechanism. Deep learning models were fed multivariate time series signals based on the raw data for each battery across the first 100 cycles. Our experiments revealed that the machine learning algorithms on handcrafted features performed particularly well, resulting in 10-20% average mean absolute percentage error. The best-performing algorithm was the Random Forest Regressor, which gave a minimum 9.8% mean absolute percentage error. Traditional machine learning models excelled due to their capability to comprehend general data set trends. In comparison, deep learning models were observed to perform particularly poorly on raw, limited data. Algorithms like GRU and RNNs that focused on capturing medium-range data dependencies were less adept at recognizing the gradual, slow trends critical for this task. Our investigation reveals that implementing machine learning models with hand-crafted features proves to be more effective than advanced deep learning models for predicting the remaining useful Lithium-ion battery life with limited data availability.

Battery degradation remains a pivotal concern in the energy storage domain, with machine learning emerging as a potent tool to drive forward insights and solutions. However, this intersection of electrochemical science and machine learning poses complex challenges. Machine learning experts often grapple with the intricacies of battery science, while battery researchers face hurdles in adapting intricate models tailored to specific datasets. Beyond this, a cohesive standard for battery degradation modeling, inclusive of data formats and evaluative benchmarks, is conspicuously absent. Recognizing these impediments, we present BatteryML - a one-step, all-encompass, and open-source platform designed to unify data preprocessing, feature extraction, and the implementation of both traditional and state-of-the-art models. This streamlined approach promises to enhance the practicality and efficiency of research applications. BatteryML seeks to fill this void, fostering an environment where experts from diverse specializations can collaboratively contribute, thus elevating the collective understanding and advancement of battery research.The code for our project is publicly available on GitHub at https://github.com/microsoft/BatteryML.

Lithium-ion batteries are widely used in various applications, including electric vehicles and renewable energy storage. The prediction of the remaining useful life (RUL) of batteries is crucial for ensuring reliable and efficient operation, as well as reducing maintenance costs. However, determining the life cycle of batteries in real-world scenarios is challenging, and existing methods have limitations in predicting the number of cycles iteratively. In addition, existing works often oversimplify the datasets, neglecting important features of the batteries such as temperature, internal resistance, and material type. To address these limitations, this paper proposes a two-stage remaining useful life prediction scheme for Lithium-ion batteries using a spatio-temporal multimodal attention network (ST-MAN). The proposed model is designed to iteratively predict the number of cycles required for the battery to reach the end of its useful life, based on available data. The proposed ST-MAN is to capture the complex spatio-temporal dependencies in the battery data, including the features that are often neglected in existing works. Experimental results demonstrate that the proposed ST-MAN model outperforms existing CNN and LSTM-based methods, achieving state-of-the-art performance in predicting the remaining useful life of Li-ion batteries. The proposed method has the potential to improve the reliability and efficiency of battery operations and is applicable in various industries, including automotive and renewable energy.

Early prediction of remaining useful life (RUL) is crucial for effective battery management across various industries, ranging from household appliances to large-scale applications. Accurate RUL prediction improves the reliability and maintainability of battery technology. However, existing methods have limitations, including assumptions of data from the same sensors or distribution, foreknowledge of the end of life (EOL), and neglect to determine the first prediction cycle (FPC) to identify the start of the unhealthy stage. This paper proposes a novel method for RUL prediction of Lithium-ion batteries. The proposed framework comprises two stages: determining the FPC using a neural network-based model to divide the degradation data into distinct health states and predicting the degradation pattern after the FPC to estimate the remaining useful life as a percentage. Experimental results demonstrate that the proposed method outperforms conventional approaches in terms of RUL prediction. Furthermore, the proposed method shows promise for real-world scenarios, providing improved accuracy and applicability for battery management.