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 li-ion battery


Survival Analysis with Machine Learning for Predicting Li-ion Battery Remaining Useful Life

arXiv.org Artificial Intelligence

The accurate prediction of RUL for lithium-ion batteries is crucial for enhancing the reliability and longevity of energy storage systems. Traditional methods for RUL prediction often struggle with issues such as data sparsity, varying battery chemistries, and the inability to capture complex degradation patterns over time. In this study, we propose a survival analysis-based framework combined with deep learning models to predict the RUL of lithium-ion batteries. Specifically, we utilize five advanced models: the Cox-type models (Cox, CoxPH, and CoxTime) and two machine-learning-based models (DeepHit and MTLR). These models address the challenges of accurate RUL estimation by transforming raw time-series battery data into survival data, including key degradation indicators such as voltage, current, and internal resistance. Advanced feature extraction techniques enhance the model's robustness in diverse real-world scenarios, including varying charging conditions and battery chemistries. Our models are tested using 10-fold cross-validation, ensuring generalizability and minimizing overfitting. Experimental results show that our survival-based framework significantly improves RUL prediction accuracy compared to traditional methods, providing a reliable tool for battery management and maintenance optimization. This study contributes to the advancement of predictive maintenance in battery technology, offering valuable insights for both researchers and industry practitioners aiming to enhance the operational lifespan of lithium-ion batteries.


Balancing SoC in Battery Cells using Safe Action Perturbations

arXiv.org Artificial Intelligence

Managing equal charge levels in active cell balancing while charging a Li-ion battery is challenging. An imbalance in charge levels affects the state of health of the battery, along with the concerns of thermal runaway and fire hazards. Traditional methods focus on safety assurance as a trade-off between safety and charging time. Others deal with battery-specific conditions to ensure safety, therefore losing on the generalization of the control strategies over various configurations of batteries. In this work, we propose a method to learn safe battery charging actions by using a safety-layer as an add-on over a Deep Reinforcement Learning (RL) agent. The safety layer perturbs the agent's action to prevent the battery from encountering unsafe or dangerous states. Further, our Deep RL framework focuses on learning a generalized policy that can be effectively employed with varying configurations of batteries. Our experimental results demonstrate that the safety-layer based action perturbation incurs fewer safety violations by avoiding unsafe states along with learning a robust policy for several battery configurations.


Improving Low-Fidelity Models of Li-ion Batteries via Hybrid Sparse Identification of Nonlinear Dynamics

arXiv.org Artificial Intelligence

Accurate modeling of lithium ion (li-ion) batteries is essential for enhancing the safety, and efficiency of electric vehicles and renewable energy systems. This paper presents a data-inspired approach for improving the fidelity of reduced-order li-ion battery models. The proposed method combines a Genetic Algorithm with Sequentially Thresholded Ridge Regression (GA-STRidge) to identify and compensate for discrepancies between a low-fidelity model (LFM) and data generated either from testing or a high-fidelity model (HFM). The hybrid model, combining physics-based and data-driven methods, is tested across different driving cycles to demonstrate the ability to significantly reduce the voltage prediction error compared to the baseline LFM, while preserving computational efficiency. The model robustness is also evaluated under various operating conditions, showing low prediction errors and high Pearson correlation coefficients for terminal voltage in unseen environments.


SambaMixer: State of Health Prediction of Li-ion Batteries using Mamba State Space Models

arXiv.org Artificial Intelligence

The state of health (SOH) of a Li-ion battery is a critical parameter that determines the remaining capacity and the remaining lifetime of the battery. In this paper, we propose SambaMixer a novel structured state space model (SSM) for predicting the state of health of Li-ion batteries. The proposed SSM is based on the MambaMixer architecture, which is designed to handle multi-variate time signals. We evaluate our model on the NASA battery discharge dataset and show that our model outperforms the state-of-the-art on this dataset. We further introduce a novel anchor-based resampling method which ensures time signals are of the expected length while also serving as augmentation technique. Finally, we condition prediction on the sample time and the cycle time difference using positional encodings to improve the performance of our model and to learn recuperation effects. Our results proof that our model is able to predict the SOH of Li-ion batteries with high accuracy and robustness.


The State of Lithium-Ion Battery Health Prognostics in the CPS Era

arXiv.org Artificial Intelligence

Lithium-ion batteries (Li-ion) have revolutionized energy storage technology, becoming integral to our daily lives by powering a diverse range of devices and applications. Their high energy density, fast power response, recyclability, and mobility advantages have made them the preferred choice for numerous sectors. This paper explores the seamless integration of Prognostics and Health Management within batteries, presenting a multidisciplinary approach that enhances the reliability, safety, and performance of these powerhouses. Remaining useful life (RUL), a critical concept in prognostics, is examined in depth, emphasizing its role in predicting component failure before it occurs. The paper reviews various RUL prediction methods, from traditional models to cutting-edge data-driven techniques. Furthermore, it highlights the paradigm shift toward deep learning architectures within the field of Li-ion battery health prognostics, elucidating the pivotal role of deep learning in addressing battery system complexities. Practical applications of PHM across industries are also explored, offering readers insights into real-world implementations.This paper serves as a comprehensive guide, catering to both researchers and practitioners in the field of Li-ion battery PHM.


De-SaTE: Denoising Self-attention Transformer Encoders for Li-ion Battery Health Prognostics

arXiv.org Artificial Intelligence

The usage of Lithium-ion (Li-ion) batteries has gained widespread popularity across various industries, from powering portable electronic devices to propelling electric vehicles and supporting energy storage systems. A central challenge in Li-ion battery reliability lies in accurately predicting their Remaining Useful Life (RUL), which is a critical measure for proactive maintenance and predictive analytics. This study presents a novel approach that harnesses the power of multiple denoising modules, each trained to address specific types of noise commonly encountered in battery data. Specifically, a denoising auto-encoder and a wavelet denoiser are used to generate encoded/decomposed representations, which are subsequently processed through dedicated self-attention transformer encoders. After extensive experimentation on NASA and CALCE data, a broad spectrum of health indicator values are estimated under a set of diverse noise patterns. The reported error metrics on these data are on par with or better than the state-of-the-art reported in recent literature.


Health diagnosis and recuperation of aged Li-ion batteries with data analytics and equivalent circuit modeling

arXiv.org Artificial Intelligence

Battery health assessment and recuperation play a crucial role in the utilization of second-life Li-ion batteries. However, due to ambiguous aging mechanisms and lack of correlations between the recovery effects and operational states, it is challenging to accurately estimate battery health and devise a clear strategy for cell rejuvenation. This paper presents aging and reconditioning experiments of 62 commercial high-energy type lithium iron phosphate (LFP) cells, which supplement existing datasets of high-power LFP cells. The relatively large-scale data allow us to use machine learning models to predict cycle life and identify important indicators of recoverable capacity. Considering cell-to-cell inconsistencies, an average test error of $16.84\% \pm 1.87\%$ (mean absolute percentage error) for cycle life prediction is achieved by gradient boosting regressor given information from the first 80 cycles. In addition, it is found that some of the recoverable lost capacity is attributed to the lateral lithium non-uniformity within the electrodes. An equivalent circuit model is built and experimentally validated to demonstrate how such non-uniformity can be accumulated, and how it can give rise to recoverable capacity loss. SHapley Additive exPlanations (SHAP) analysis also reveals that battery operation history significantly affects the capacity recovery.


Physics-Informed Neural Networks for Prognostics and Health Management of Lithium-Ion Batteries

arXiv.org Artificial Intelligence

For Prognostics and Health Management (PHM) of Lithium-ion (Li-ion) batteries, many models have been established to characterize their degradation process. The existing empirical or physical models can reveal important information regarding the degradation dynamics. However, there are no general and flexible methods to fuse the information represented by those models. Physics-Informed Neural Network (PINN) is an efficient tool to fuse empirical or physical dynamic models with data-driven models. To take full advantage of various information sources, we propose a model fusion scheme based on PINN. It is implemented by developing a semi-empirical semi-physical Partial Differential Equation (PDE) to model the degradation dynamics of Li-ion batteries. When there is little prior knowledge about the dynamics, we leverage the data-driven Deep Hidden Physics Model (DeepHPM) to discover the underlying governing dynamic models. The uncovered dynamics information is then fused with that mined by the surrogate neural network in the PINN framework. Moreover, an uncertainty-based adaptive weighting method is employed to balance the multiple learning tasks when training the PINN. The proposed methods are verified on a public dataset of Li-ion Phosphate (LFP)/graphite batteries.


A Deep Learning Approach Towards Generating High-fidelity Diverse Synthetic Battery Datasets

arXiv.org Artificial Intelligence

Recent surge in the number of Electric Vehicles have created a need to develop inexpensive energy-dense Battery Storage Systems. Many countries across the planet have put in place concrete measures to reduce and subsequently limit the number of vehicles powered by fossil fuels. Lithium-ion based batteries are presently dominating the electric automotive sector. Energy research efforts are also focussed on accurate computation of State-of-Charge of such batteries to provide reliable vehicle range estimates. Although such estimation algorithms provide precise estimates, all such techniques available in literature presume availability of superior quality battery datasets. In reality, gaining access to proprietary battery usage datasets is very tough for battery scientists. Moreover, open access datasets lack the diverse battery charge/discharge patterns needed to build generalized models. Curating battery measurement data is time consuming and needs expensive equipment. To surmount such limited data scenarios, we introduce few Deep Learning-based methods to synthesize high-fidelity battery datasets, these augmented synthetic datasets will help battery researchers build better estimation models in the presence of limited data. We have released the code and dataset used in the present approach to generate synthetic data. The battery data augmentation techniques introduced here will alleviate limited battery dataset challenges.


Machine Learning-Aided Discovery of Superionic Solid-State Electrolyte for Li-Ion Batteries

arXiv.org Artificial Intelligence

Li-Ion Solid-State Electrolytes (Li-SSEs) are a promising solution that resolves the critical issues of conventional Li-Ion Batteries (LIBs) such as poor ionic conductivity, interfacial instability, and dendrites growth. In this study, a platform consisting of a high-throughput screening and a machine-learning surrogate model for discovering superionic Li-SSEs among 20,237 Li-containing materials is developed. For the training database, the ionic conductivity of Na SuperIonic CONductor (NASICON) and Li SuperIonic CONductor (LISICON) type SSEs are obtained from the previous literature. Then, the chemical descriptor (CD) and additional structural properties are used as machine-readable features. Li-SSE candidates are selected through the screening criteria, and the prediction on the ionic conductivity of those is followed. Then, to reduce uncertainty in the surrogate model, the ensemble method by considering the best-performing two models is employed, whose mean prediction accuracy is 0.843 and 0.829, respectively. Furthermore, first-principles calculations are conducted for confirming the ionic conductivity of the strong candidates. Finally, six potential superionic Li-SSEs that have not previously been investigated are proposed. We believe that the constructed platform can accelerate the search for Li-SSEs with high ionic conductivity at minimum cost.